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Program Scientific Program
POS5-1354

Antisolvent Engineering with Small Molecule Additives for Efficient and Stable Near-Infrared Perovskite Light-Emitting Diodes

When and Where

Nov 30, -0001   00:00 - 00:00

Presenter(s)

Seungwoo Song (Gwangju Institute of Science and Technology (GIST))

Co-Author(s)

Hobeom Kim (Gwangju Institute of Science and Technology (GIST)), Dongbeen Lee (Gwangju Institute of Science and Technology (GIST)), ByungJun Yoo (Gwangju Institute of Science and Technology (GIST)), Sang-Jeung Park (Gwangju Institute of Science and Technology (GIST)), Yeonji Son (Gwangju Institute of Science and Technology (GIST)), Junmo Park (Gwangju Institute of Science and Technology (GIST))

Abstract

Formamidinium lead iodide (FAPbI₃) is widely studied as a near-infrared emitter for perovskite light-emitting diodes (NIR PeLEDs) owing to its narrow bandgap and favorable optoelectronic properties. Nevertheless, defects in FAPbI₃ films form trap states that induce non-radiative recombination and facilitate ion migration, leading to reduced device efficiency and structural instability. Here, we employ an antisolvent-assisted strategy to induce rapid nucleation during film formation, yielding dense and uniform perovskite films. Small-molecule additives incorporated into the antisolvent may interact with undercoordinated Pb²⁺ sites, possibly enabling effective defect passivation. Consequently, the optimized devices achieved a peak external quantum efficiency (EQE) of 10.8%, compared with 6.5% for the control device. These results indicate that incorporating small-molecule additives into the antisolvent is an effective approach for suppressing non-radiative recombination and improving the performance of FAPbI₃-based NIR PeLEDs.

Acknowledgements
This research was supported by the National Research Foundation of Korea (NRF) grant funded by the Korea government (MSIT) (RS-2024-00342991). This research was supported by the National Research Foundation of Korea(NRF) grant funded by the Korea government (MSIT) (RS-2024-00437887). This research was supported by Korea Basic Science Institute(National research Facilities and Equipment Center) grant funded by the Ministry of Science and ICT (RS-2026-25500164). This research was supported by the Digital Research Innovation Institution Program through the National Research Foundation of Korea (NRF) funded by Ministry of Science and ICT (RS-2023-00283597).
Supported by
Korea Tourism Organization BUSAN TOURISM ORGANIZATION
Sponsored by
Korea Research Institute of Chemical Technology Advanced Materials Division Sejin CI DONGJIN SEMICHEM HAEDONG SCIENCE FOUNDATION COSMAX EcoProBM Young Eng. Sci. Doosan SAMSUNG SDI S-OIL 한국도레이과학진흥재단