Two-Dimensional Fused Aromatic Network Polymers as Electrocatalytic Platforms
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Two-dimensional fused aromatic network polymers have attracted immense interest, because of their electronic, optoelectronic, magnetic and electrocatalytic properties. Their tunable structures and properties promise to offer many opportunities in various practical applications. However, even after years of intensive researches in science and technology, facile and scalable methods capable of producing robust fused-aromatic network polymers, composed of periodic holes with uniformly decorated heteroatoms, remain very limited. Here, ultrastable fused aromatic network polymers have been designed and synthesized as platforms for anchoring metal nanoclusters and nanoparticles to form efficient electrocatalysts (Figure 1).1-4 (1) Mahmood, et al.. Nat. Commun., 6, 6486 (2015). (2) Mahmood, et al., Nat. Nanotechnol., 12, 441 (2017). (3) Seo et al., J. Am. Chem. Soc., 141, 11786 (2019). (4) Seo et al., J. Am. Chem. Soc., 144, 19973 (2022).